Aufsatz
Observation of a Long-lived Electronic Coherence Modulated by Vibrational Dynamics in Molecular Nd³+- Complexes at Room Temperature
Abstract
Temporally delayed, phase-locked coherent pairs of near IR femtosecond laser pulses were employed to study electronic coherences in molecular Nd³+-complexes at room temperature. Dissolved and solid complexes were studied under a confocal microscope set-up with fluorescence detection. The observed electronic coherence on a few hundred femtoseconds time scale is modulated by additional coherent wave packet dynamics, which we attribute mainly to be vibrational in nature. In future, the complexes may serve as prototypes for possible applications in quantum information technology.
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Gefördert im Rahmen des Projekts DEALCitation
@article{doi:10.17170/kobra-202307248458,
author={Ghosh, Jayanta and Gheibi, Mirali and Kalas, Tillmann and Sarpe, Cristian and Zielinski, Bastian and Ciobotea, Ramela and Morscher, Christoph Burghard and Koehne, Ingo and Pietschnig, Rudolf and Senftleben, Arne and Baumert, Thomas and Braun, Hendrike},
title={Observation of a Long-lived Electronic Coherence Modulated by Vibrational Dynamics in Molecular Nd³+- Complexes at Room Temperature},
journal={ChemPhysChem},
year={2023}
}
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3000 Ghosh, Jayanta
3010 Gheibi, Mirali
3010 Kalas, Tillmann
3010 Sarpe, Cristian
3010 Zielinski, Bastian
3010 Ciobotea, Ramela
3010 Morscher, Christoph Burghard
3010 Koehne, Ingo
3010 Pietschnig, Rudolf
3010 Senftleben, Arne
3010 Baumert, Thomas
3010 Braun, Hendrike
4000 Observation of a Long-lived Electronic Coherence Modulated by Vibrational Dynamics in Molecular Nd³+- Complexes at Room Temperature / Ghosh, Jayanta
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