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Dissertation

Optimal Control of Quantum Information Tasks in Open Quantum Systems
(2020-07-30)
Every quantum system inevitably interacts with its environment. This is a fundamental requirement that allows us to control, measure and, in general, interact with quantum systems. In that respect, a quantum system's openness can be interpreted as prerequisite that enables quantum technologies in the first place. The latter are built to harness the intrinsic quantum mechanical behavior of quantum devices in order to build new, powerful technologies. However, a quantum system's openness also causes it to interact ...
Dissertation

Gold Surface Nanostructuring with Ultrashort Laser Pulses - Study of Non-equilibrium Effects
(2019)
Laser material interaction and structure formation in metals under controlled ultrashort laser pulse conditions are discussed in this work. A novel approach is presented describing the exact amount of energy deposited by a laser pulse in a gold surface, applicable under a variety of structuring conditions. The presented model is validated by a new introduced broad-band pump-probe reflectivity measurement method. A technique also applicable to investigate other phenomenas where 20 fs resolution combined with an octave ...
Dissertation
Bestimmung der mittleren Clustergröße und ortsspezifischen Zustände homogener Edelgascluster mittels Fluoreszenzspektroskopie
(2021)
Der Übergang von mikroskopischen zu makroskopischen Systemen ist in den Naturwissenschaften von grundlegendem Interesse, da im zugehörigen Übergangsbereich größenabhängige Entwicklungen physikalischer Eigenschaften sowie auch gänzlich neue Prozesse auftreten. Edelgascluster ermöglichen einen experimentellen Zugang zur Untersuchung dieses Zwischenbereichs.
Die durch Van-der-Waals-Kräfte gebundenen inerten Edelgasatome fungieren als Prototypsysteme zur Untersuchung derartiger fundamentaler Prozesse. Sie werden mittels ...
Dissertation

Electron Dynamics Driven by Intense Coherent Femtosecond Laser Pulses: Dynamic Interference in Atoms and Photoelectron Circular Dichroism in Chiral Molecules
(2018-12)
Since humans have begun to explore nature, they came up with new ways and tools, which
have been permanently improved. At some point, those tools allowed to look into the
microworld and to study the quantum nature of matter. One of such tools to explore the
quantum world is the light amplification by stimulated emission of radiation (laser). Since the
first lasers were built almost 60 years ago, their capabilities improved permanently, allowing
the study of hitherto-unknown physical phenomena. Two of such ...
Dissertation

Visualizing the electronic structure of small molecules with rovibronic photon emission spectroscopy
(2018)
A key in understanding the fundamental structure of atoms and molecules has been their absorption and emission of electromagnetic radiation across all spectral ranges. The observation of discrete line spectra contributed to the development of core concepts in quantum mechanics and thus the modern picture of physical processes occurring at small scales. The ongoing refinement of both experimental and theoretical methods in spectroscopy allows to deal with succeedingly more complex systems in different interactions to ...
Dissertation

High-Speed 1.55 µm Quantum Dot Lasers with Electronically Coupled Quantum Well - Dot Active Regions
(2019-07-31)
The expansion of long-distance data communication at a wavelength of 1.55 µm calls for larger data transfer rates. Consequently, an improvement of emission and modulation properties of lasers emitting in this wavelength region is of high interest. The utilization of so-called tunnel-injection (TI) structures in InP-based quantum dot (QD) lasers is promising to fulfill this task. The aim of this thesis was the realization and analysis of TI structures in the lattice matched InP material system and incorporation into ...
Dissertation
Quantum optimal control theory of photoelectron spectroscopy
(2018)
The object of this doctoral thesis is two-fold and can be classified into two, but intrinsically related categories: (i) development of theoretical models for the simulation of electron dynamics and in parallel to this, (ii) method development of efficient numerical algorithms for ad hoc control of photoelectron and photoion-related observables. The first category primarily focuses on the development of a variety of theoretical models describing the interaction of light and matter for the extraction and control of ...
Dissertation

1.55 μm Quantum Dot Lasers for Telecommunication
(2019)
The thesis at hand investigates the suitability of quantum dot (QD) material for use in long-distance coherent communication. The thesis was written in the frame of the SASER project MONOLOP that is aiming for a compact, monolithically integrated light source with a tunable wavelength covering the C+-band and narrow spectral linewidth below 500 kHz.
The thesis reviews the theoretical background of quantum dot material based on the InP material system and distributed feedback (DFB) lasers with lateral gratings as ...
Dissertation

Development of Carrier-Envelope-Phase-Stabilized, mJ-Class Laser Sources Generating Intense, Few-Cycle Laser Pulses
(2020-05-19)
Over a decade ago the frontiers of ultrashort physics and nonlinear optics have reached the attosecond timescale ($1 as = 10 ^ {-18} s$) . Currently, in order to generate isolated attosecond pulses, an intense femtosecond pulse is focused in a jet of a noble gas. Given the sufficient intensity, this leads to high harmonic generation (HHG), which can be filtered (gated) to create a single isolated attosecond pulse. The laser source for the driver pulses has to fulfill two requirements: the pulses need to be limited ...