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High-Purity Triggered Single-Photon Emission from Symmetric Single InAs/InP Quantum Dots around the Telecom C-Band Window
(2019-11-07)
The authors demonstrate pure triggered single‐photon emission from quantum dots (QDs) around the telecommunication C‐band window, with characteristics preserved under non‐resonant excitation at saturation, that is, the highest possible, lifetime‐limited emission rates. The direct measurement of emission dynamics reveals photoluminescence decay times in the range of (1.7–1.8) ns corresponding to maximal photon generation rates exceeding 0.5 GHz. The measurements of the second‐order correlation function exhibit, for ...
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Temporal Airy pulses for controlled high aspect ratio nanomachining of dielectrics
(2016-04-05)
Understanding the interplay between optical pulse parameters and ultrafast material response is critical in achieving efficient and controlled laser nanomachining. In general, the key to initiate material processing is the deposition of a sufficient energy density within the electronic system. In dielectrics this critical energy density corresponds typically to a plasma frequency in the near-IR spectral region. Creating this density instantaneously with ultrashort laser pulses of a few tens of femtoseconds pulse ...
Aufsatz
Tunneling Time in Attosecond Experiments and Time Operator in Quantum Mechanics
(2018-10-08)
Attosecond science is of a fundamental interest in physics. The measurement of the tunneling time in attosecond experiments, offers a fruitful opportunity to understand the role of time in quantum mechanics (QM). We discuss in this paper our tunneling time model in relation to two time operator definitions introduced by Bauer and Aharonov–Bohm. We found that both definitions can be generalized to the same type of time operator. Moreover, we found that the introduction of a phenomenological parameter by Bauer to fit ...
Aufsatz
Beating the limits with initial correlations
(2017-11-28)
Fast and reliable reset of a qubit is a key prerequisite for any quantum technology. For real world open quantum systems undergoing non-Markovian dynamics, reset implies not only purification, but in particular erasure of initial correlations between qubit and environment. Here, we derive optimal reset protocols using a combination of geometric and numerical control theory. For factorizing initial states, we find a lower limit for the entropy reduction of the qubit as well as a speed limit. The time-optimal solution ...
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A simulation-based approach to evaluate objective material parameters from concrete rheometer measurements
(2019-12-31)
Modern concretes such as ultra-high performance concrete (UHPC) show excellent strength properties combined with favorable flow properties. However, the flow properties depend strongly on process parameters during production (temperature, humidity etc.), but also change sensitively even with slight variations in the mixture. In order to ensure desired processing of the fluidlike material and consistent process quality, the flow properties of the concrete must be evaluated quantitatively and objectively. The usual ...
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Numerical Investigation of Ultrashort Laser-Ablative Synthesis of Metal Nanoparticles in Liquids Using the Atomistic-Continuum Model
(2019-12-24)
We present a framework based on the atomistic continuum model, combining the Molecular Dynamics (MD) and Two Temperature Model (TTM) approaches, to characterize the growth of metal nanoparticles (NPs) under ultrashort laser ablation from a solid target in water ambient. The model is capable of addressing the kinetics of fast non-equilibrium laser-induced phase transition processes at atomic resolution, while in continuum it accounts for the effect of free carriers, playing a determinant role during short laser pulse ...
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Electronic origin of bond softening and hardening in femtosecond-laser-excited magnesium
(IOP, 2014)
Many ultrafast structural phenomena in solids at high fluences are related to the hardening or softening of particular lattice vibrations at lower fluences. In this paper we relate femtosecond-laser-induced phonon frequency changes to changes in the electronic density of states, which need to be evaluated only in the electronic ground state, following phonon displacement patterns. We illustrate this relationship for a particular lattice vibration of magnesium, for which we—surprisingly—find that there is both softening ...
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Controlling the transport of an ion: classical and quantum mechanical solutions
(IOP, 2014)
The accurate transport of an ion over macroscopic distances represents a challenging control problem due to the different length and time scales that enter and the experimental limitations on the controls that need to be accounted for. Here, we investigate the performance of different control techniques for ion transport in state-of-the-art segmented miniaturized ion traps. We employ numerical optimization of classical trajectories and quantum wavepacket propagation as well as analytical solutions derived from invariant ...
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Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters
(2018-01-16)
We directly observe radiative charge transfer (RCT) in Ne clusters by dispersed vacuum-ultraviolet photon detection. The doubly ionized Ne^2+ – Ne_n-1 initial states of RCT are populated after resonant 1s–3p photoexcitation or 1s photoionization of Ne_n clusters with {n} \approx 2800. These states relax further producing Ne^+ – Ne^+ – Ne_n-2 final states, and the RCT photon is emitted. Ab initio calculations assign the observed RCT signal to the Ne^2+(2p^-2 [^1D]) - Ne_n-1 initial state, while transitions from other ...
Aufsatz
Reservoir engineering using quantum optimal control for qubit reset
(2019-09-24)
We determine how to optimally reset a superconducting qubit which interacts with a thermal environment in such a way that the coupling strength is tunable. Describing the system in terms of a time-local master equation with time-dependent decay rates and using quantum optimal control theory, we identify temporal shapes of tunable level splittings which maximize the efficiency of the reset protocol in terms of duration and error. Time-dependent level splittings imply a modification of the system-environment coupling, ...