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Theoretical study of spin polarization in multiphoton ionization of Xe
Abstract
Spin polarization in the multiphoton above-threshold ionization of 5p3/2- and 5p1/2-electrons of Xe with intense 395nm, circularly polarized laser pulses, is investigated theoretically. For this purpose, we solve the time-dependent Schrödinger equation on the basis of spherical spinors. We, thus, simultaneously propagate the spin-up and spin-down single-active-electron wave packets, driven by the laser pulses in the ionic potential, which includes the spin–orbit interaction explicitly. The present theoretical results are in good agreement with the recent experimental results
Citation
In: The Journal of Chemical Physics Volume 158 / Issue 15 (2023-04-21) eissn:1089-7690Sponsorship
Gefördert im Rahmen des Projekts DEALCitation
@article{doi:10.17170/kobra-202305198053,
author={Artemyev, Anton N. and Kutscher, Eric and Lagutin, Boris M. and Demekhin, Philipp V.},
title={Theoretical study of spin polarization in multiphoton ionization of Xe},
journal={The Journal of Chemical Physics},
year={2023}
}
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2023-05-19T08:34:56Z 2023-05-19T08:34:56Z 2023-04-21 doi:10.17170/kobra-202305198053 http://hdl.handle.net/123456789/14724 Gefördert im Rahmen des Projekts DEAL eng Namensnennung 4.0 International http://creativecommons.org/licenses/by/4.0/ 530 540 Theoretical study of spin polarization in multiphoton ionization of Xe Aufsatz Spin polarization in the multiphoton above-threshold ionization of 5p3/2- and 5p1/2-electrons of Xe with intense 395nm, circularly polarized laser pulses, is investigated theoretically. For this purpose, we solve the time-dependent Schrödinger equation on the basis of spherical spinors. We, thus, simultaneously propagate the spin-up and spin-down single-active-electron wave packets, driven by the laser pulses in the ionic potential, which includes the spin–orbit interaction explicitly. The present theoretical results are in good agreement with the recent experimental results open access Artemyev, Anton N. Kutscher, Eric Lagutin, Boris M. Demekhin, Philipp V. 6 Seiten doi:10.1063/5.0142679 Spinpolarisation Mehrphotonenprozess Xenon publishedVersion eissn:1089-7690 Issue 15 The Journal of Chemical Physics Volume 158 false 154115
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