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Aufsatz
On the total energy of two-electron atoms
(1985)
Using the Multi-Configuration Dirac-Fock (MCDF) method we calculate with 9 configuration state functions the correlation energy as well as the total energy of the lowest J = 0 ground state of all two-electron systems from H- to Thorium (Z = 90). A comparison with experimental data, which are available only in the low Z region, shows a very good agreement.
Aufsatz
Atomic and ionic radii of superheavy elements
(1972)
Atomic and ionic radii are presented for the elements E104-E120 and E156-E172. It is shown that a number of effects correlated with the large relativistic contraction of orbitals with low angular momentum leads to smaller atoms for higher atomic numbers. It is expected that Cs is the largest atom in nature.
Aufsatz
{2p_\pi}-{2p_\sigma} crossing in heavy symmetric ion-atom collisions: I. Level structure
(1982)
Ab initio self-consistent DFS calculations are performed for five different symmetric
atomic systems from Ar-Ar to Pb-Pb. The level structure for the {2p_\pi}-{2p_\sigma} crossing as function of the united atomic charge Z_u is studied and interpreted. Manybody effects, spin-orbit splitting, direct relativistic effects as well as indirect relativistic effects are differently important for different Z_u. For the I-I system a comparison with other calculations is given.
Aufsatz
Many-electron relativistic calculation and interpretation of atomic processes in time dependent heavy-ion scattering
(1989)
The time dependence of a heavy-ion-atom collision system is solved via a set of coupled channel equations using energy eigenvalues and matrix elements from a self-consistent field relativistic molecular many-electron Dirac-Fock-Slater calculation. Within this independent particle model we give a full many-particle interpretation by performing a small number of single-particle calculations.
First results for the P(b) curves for the Ne K-hole excitation for the systems F{^8+} - Ne and F{^6+} - Ne as examples are discussed.
Aufsatz
Femtosecond pump-probe study of the spreading and recurrence of a vibrational wave packet in Na_2
(1992)
The motion of a vibrational wave packet in the bound A(^1 \summe^+_u) electronic state of the sodium dimer is detected in a femtosecond pump/probe molecular beam experiment. For short times harmonic motion is seen in the total ion yield of Na^+_2 as a function of delay time between the two laser pulses. The spreading of the wave packet results in the loss of the periodic variation of the ion signal. For longer delay times (47 ps) the wave packet regains its initial form which is reflected in the revival structure of ...
Aufsatz
Autoionization and fragmentation of Na_2 studied by femtosecond laser pulses
(Ed. by Michael S. Feld u.a., 1989)