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Dissertation
Quantum optimal control theory of photoelectron spectroscopy
(2018)
The object of this doctoral thesis is two-fold and can be classified into two, but intrinsically related categories: (i) development of theoretical models for the simulation of electron dynamics and in parallel to this, (ii) method development of efficient numerical algorithms for ad hoc control of photoelectron and photoion-related observables. The first category primarily focuses on the development of a variety of theoretical models describing the interaction of light and matter for the extraction and control of ...
Dissertation
Automatic computation of continued fraction representations as solutions of explicit differential equations
(2019)
The main focus of this thesis is to present a variation of an algorithm first presented by Maulat and Salvy, with which it is possible to algorithmically guess as well as prove continued fraction expansions of analytical expressions with the help of ordinary differential equations.
Dissertation
Gold Surface Nanostructuring with Ultrashort Laser Pulses - Study of Non-equilibrium Effects
(2019)
Laser material interaction and structure formation in metals under controlled ultrashort laser pulse conditions are discussed in this work. A novel approach is presented describing the exact amount of energy deposited by a laser pulse in a gold surface, applicable under a variety of structuring conditions. The presented model is validated by a new introduced broad-band pump-probe reflectivity measurement method. A technique also applicable to investigate other phenomenas where 20 fs resolution combined with an octave ...
Aufsatz
Role of Pseudouridine Formation by Deg1 for Functionality of Two Glutamine Isoacceptor tRNAs
(2017-01-26)
Loss of Deg1/Pus3 and concomitant elimination of pseudouridine in tRNA at positions 38 and 39 (ψ38/39) was shown to specifically impair the function of tRNAGlnUUG under conditions of temperature-induced down-regulation of wobble uridine thiolation in budding yeast and is linked to intellectual disability in humans. To further characterize the differential importance of the frequent ψ38/39 modification for tRNAs in yeast, we analyzed the in vivo function of non-sense suppressor tRNAs SUP4 and sup70-65 in the absence ...
Dissertation
Das Reaktionsverhalten N-heterocyclischer Plumbylene mit 1,1'-Ferrocendiyl-Rückgrat
(2020-10)
Dieses Dissertationsprojekt befasst sich mit dem Reaktionsverhalten von cyclischen Diaminoplumbylenen mit 1,1‘-Ferrocendiyl-Rückgat. Die zugrunde liegende Fragestellung entstand, nachdem im Jahr 2010 ein analoges N-heterocyclisches Carben (NHC) durch sein besonderes Reaktionsverhalten für Aufsehen sorgte, denn dieses ist beispielsweise dazu in der Lage mit Kohlenstoffmonoxid zu reagieren, was von einer besonders ausgeprägten Ambiphilie zeugt und in der Stoffklasse der NHC beispiellos ist. Ob schwere Analoga dieses ...
Dissertation
Ab-initio analysis of the structural response of solids after femtosecond-laser-pulse excitation
(2019)
After an intense femtosecond-laser excitation extreme non-equilibrium conditions are induced in materials. The high photon density in such an ultrashort-laser pulse interacts directly with the electronic system of the material. By absorbing the photon energy the electrons are excited in high energy states, where they form a non-equilibrium distribution shortly after the excitation. Due to fast electron-electron scattering and cascading processes equilibrates the electronic system within several femtoseconds to a ...
Dissertation
InP - based quantum dots for telecom wavelengths ranges
(2019-12)
Long-distance quantum communication applications require sources of single photons, emitting at telecom wavelengths (around 1550 nm) with minimum attenu-ation losses of silica fiber.
Semiconductor self-assembled InAs/InP-based quantum dots (QDs) are possible candidates to
reach this spectral region. One of the challenges on the way is a QD asymmetry, which limits the fidelity of entangled photons. Therefore, morphological and optical properties of QDs should be improved in order to achieve the necessary quality and ...
Dissertation
Abhängigkeit des Exchange-Bias Feldes und des Koerzitivfeldes von der mittels Röntgendiffraktometrie gemessenen Kornvolumenverteilung des Antiferromagneten in Exchange-Bias Schichtsystemen
(2019-10-02)
Der Exchange-Bias Effekt wird in vielen technischen Anwendungen, wie z.B. in magnetischen Speichermedien oder in Magnetsensorköpfen zum Pinnen der Magnetisierungsrichtung der Referenzelektrode, eingesetzt. Dieser Effekt tritt ausschließlich in dünnen Schichtsystemen, in denen sich ein dünner Ferromagnet mit einem dünnen Antiferromagneten in Kontakt befindet, auf und bewirkt eine Verschiebung der Hysteresekurve entlang der Magnetfeldachse. Solche Exchange-Bias Schichtsysteme können mittels Ionenbeschuss, d.h., leichte ...
Dissertation
Role of neurotransmitter GABA in the brain of the Madeira cockroach Rhyparobia maderae with focus on the circadian system
(2019-02)
All living things are subject to biological rhythms. Circadian rhythms are generated by internal clocks which influence many biochemical and physiological processes, as well as various behaviors of an organism. These oscillators are synchronized by external "Zeitgeber" signals such as light-dark changes, temperature changes, as well as social contacts. Different studies identified the accessory medulla (AME), small neuropil at the ventromedian edge of the medulla, as the circadian pacemaker center of the cockroach ...
Aufsatz
Electronic origin of bond softening and hardening in femtosecond-laser-excited magnesium
(IOP, 2014)
Many ultrafast structural phenomena in solids at high fluences are related to the hardening or softening of particular lattice vibrations at lower fluences. In this paper we relate femtosecond-laser-induced phonon frequency changes to changes in the electronic density of states, which need to be evaluated only in the electronic ground state, following phonon displacement patterns. We illustrate this relationship for a particular lattice vibration of magnesium, for which we—surprisingly—find that there is both softening ...