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Dissertation
Gold Surface Nanostructuring with Ultrashort Laser Pulses - Study of Non-equilibrium Effects
(2019)
Laser material interaction and structure formation in metals under controlled ultrashort laser pulse conditions are discussed in this work. A novel approach is presented describing the exact amount of energy deposited by a laser pulse in a gold surface, applicable under a variety of structuring conditions. The presented model is validated by a new introduced broad-band pump-probe reflectivity measurement method. A technique also applicable to investigate other phenomenas where 20 fs resolution combined with an octave ...
Dissertation
Bestimmung der mittleren Clustergröße und ortsspezifischen Zustände homogener Edelgascluster mittels Fluoreszenzspektroskopie
(2021)
Der Übergang von mikroskopischen zu makroskopischen Systemen ist in den Naturwissenschaften von grundlegendem Interesse, da im zugehörigen Übergangsbereich größenabhängige Entwicklungen physikalischer Eigenschaften sowie auch gänzlich neue Prozesse auftreten. Edelgascluster ermöglichen einen experimentellen Zugang zur Untersuchung dieses Zwischenbereichs.
Die durch Van-der-Waals-Kräfte gebundenen inerten Edelgasatome fungieren als Prototypsysteme zur Untersuchung derartiger fundamentaler Prozesse. Sie werden mittels ...
Dissertation
High-Speed 1.55 µm Quantum Dot Lasers with Electronically Coupled Quantum Well - Dot Active Regions
(2019-07-31)
The expansion of long-distance data communication at a wavelength of 1.55 µm calls for larger data transfer rates. Consequently, an improvement of emission and modulation properties of lasers emitting in this wavelength region is of high interest. The utilization of so-called tunnel-injection (TI) structures in InP-based quantum dot (QD) lasers is promising to fulfill this task. The aim of this thesis was the realization and analysis of TI structures in the lattice matched InP material system and incorporation into ...
Dissertation
Quantum optimal control theory of photoelectron spectroscopy
(2018)
The object of this doctoral thesis is two-fold and can be classified into two, but intrinsically related categories: (i) development of theoretical models for the simulation of electron dynamics and in parallel to this, (ii) method development of efficient numerical algorithms for ad hoc control of photoelectron and photoion-related observables. The first category primarily focuses on the development of a variety of theoretical models describing the interaction of light and matter for the extraction and control of ...
Dissertation
1.55 μm Quantum Dot Lasers for Telecommunication
(2019)
The thesis at hand investigates the suitability of quantum dot (QD) material for use in long-distance coherent communication. The thesis was written in the frame of the SASER project MONOLOP that is aiming for a compact, monolithically integrated light source with a tunable wavelength covering the C+-band and narrow spectral linewidth below 500 kHz.
The thesis reviews the theoretical background of quantum dot material based on the InP material system and distributed feedback (DFB) lasers with lateral gratings as ...
Dissertation
Development of Carrier-Envelope-Phase-Stabilized, mJ-Class Laser Sources Generating Intense, Few-Cycle Laser Pulses
(2020-05-19)
Over a decade ago the frontiers of ultrashort physics and nonlinear optics have reached the attosecond timescale ($1 as = 10 ^ {-18} s$) . Currently, in order to generate isolated attosecond pulses, an intense femtosecond pulse is focused in a jet of a noble gas. Given the sufficient intensity, this leads to high harmonic generation (HHG), which can be filtered (gated) to create a single isolated attosecond pulse. The laser source for the driver pulses has to fulfill two requirements: the pulses need to be limited ...
Dissertation
Chiral recognition in the gas phase using femtosecond to nanosecond photoelectron circular dichroism
(2020-05)
Diese Arbeit konzentriert sich auf die chirale Erkennung in der Gasphase unter Verwendung der resonant verstärkten Multi-Photonen-Ionisation. Gasphasentechniken bieten die Möglichkeit, die Chiralität von Molekülen innerhalb einer nahezu interaktionsfreien Umgebung zu untersuchen. Photoionisation von chiralen Molekülen mit zirkular polarisiertem Licht führt zu einer Asymmetrie in der Photoelektronenemission bezüglich der Ausbreitungsrichtung des ionisierenden Lichts. Diese Asymmetrie ist bekannt als Photoelektronenz ...
Aufsatz
Preferential weakening of rotational magnetic anisotropy by keV-He ion bombardment in polycrystalline exchange bias layer systems
(2018-05-04)
The consequences of keV light-ion bombardment of polycrystalline exchange bias layer systems on individual magnetic anisotropies composing the effective unidirectional magnetic anisotropy are investigated by vectorial magneto-optic Kerr effect measurements. Preferential reduction of rotatable magnetic anisotropy as compared to the other magnetic anisotropies is observable, disproving the intuitive assumption of an equable weakening of all magnetic anisotropies due to the bombardment. It is concluded that light-ion ...
Dissertation
Investigation of diamond nanostructures with incorporated color centers
(2018)
Diamond is a material with excellent properties due to its structure and composition. Its crystal lattice is a perfect host of different defect centers, so-called color centers, whose properties, especially the capability of emitting single photons, can serve in quantum information technologies (QIT). As a high refractive index material only a small part of the photons emitted by these color centers in diamond can be collected. To enhance the photon collection efficiency photonic structures are necessary. They can ...