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Aufsatz
Calculation of isomer shift in Mössbauer spectroscopy
(1972)
The approximations normally used in the calculation of the isomer shift are compared with the exact expressions using Dirac-Slater orbitals and a three-parameter Fermi-type nuclear charge distribution. The nonuniformity of the electronic density over the nuclear volume affects the results. Different choices of the nuclear surface thickness t and the radius c in the protonic
density P_N (\gamma) also affects the isomer shift differently even though the values are chosen to yield a given value of \delta <r^2>. The ...
Aufsatz
The Li-like KLL-Auger spectrum of foil excitation Ne-projectiles
(1977)
KLL-Auger transitions of the three electron system in Ne have been recorded in a coincidence experiment frec of
contaminants from other systems. Energies as well as intensities are compared with calculated values.
Aufsatz
Precision laser spectroscopy of the ground state hyperfine splitting of hydrogenlike ^209 Bi^82+
(1994)
The first direct observation of a hyperfine splitting in the optical regime is reported. The wavelength of the M1 transition between the F = 4 and F = 5 hyperfine levels of the ground state of hydrogenlike ^209 Bi^82+ was measured to be \lamda_0 = 243.87(4) nm by detection of laser induced fluorescence at the heavy-ion storage ring ESR at GSI. In addition, the lifetime of the laser excited F = 5 sublevel was determined to be \tau_0 = 0.351(16) ms. The method can be applied to a number of other nuclei and should allow ...
Aufsatz
Relativity and screening effects in heavy-ion collisions
(1975)
Diatomic correlation diagrams are the main basis for the description of heavy-ion collisions. We have constructed the first realistic relativistic many-electron correlation diagrams based on nonrelativistic self-consistent-field, Hartree-Fock calculations of diatomic molecules plus relativistic corrections. We discuss the relativistic influences as well as the many-electron screening effects in the I-Au system with a combined charge of Z = 132 as an example.
Aufsatz
Precise calculations of atomic electron binding energies in fermium
(1972)
The comparison between the experimental binding energies for the K, L, and M electrons for fermium and the results of our Dirac-Fock calculation, taking into account all tractable corrections, leads to agreement within about 20 eV. This shows that the present method of calculation is an adequate description of this problem and that nonlinear electrodynamical effects will not be present in nature or will be smaller than 1% compared to the values recently proposed. It is found that the energies of electronic transitions ...
Aufsatz
On the correlation between electric polarizabilities and the ionization potential of atoms
(1985)
It is found that the electric dipole polarizabilities of neutral atoms correlate very strongly with their first ionization potential within the groups of elements with the same angular momenta of the outermost electrons. As the latter values are known very accurately, this allows a very good
(<30%) prediction of various atomic polarizabilities.
Aufsatz
Relativistic calculations of super heavy quasi-molecules
(Malli, G. L. (Hrsg.), 1983)
Aufsatz
Double-autoionization decay of resonantly excited single-electron states
(1993)
Perturbation theory in the lowest non-vanishing order in interelectron interaction has been applied to the theoretical investigation of double-ionization decays of resonantly excited single-electron states. The formulae for the transition probabilities were derived in the LS coupling scheme, and the orbital angular momentum and spin selection rules were obtained. In addition to the formulae, which are exact in this order, three approximate expressions, which correspond to illustrative model mechanisms of the transition, ...