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Aufsatz
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Experimental investigations of viscoelastic and ferroelectric heating in PZT–5H
(2021-01-25)
This contribution focuses on the separation of two effects causing a temperature change in experiments with electrically loaded ferroelectrics. These materials are often subjected to cyclic loading, where viscoelasticity prevails at lower electric fields, whereas dissipative heating by domain switching governs the heating above the coercive field. Different frequencies and load amplitudes are investigated experimentally.
Aufsatz
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Discriminatory resonance energy transfer mediated by a chiral environment
(2024-05-07)
In this study, we delve into the crucial influence of and enhancement by chiral environments on the discriminatory capabilities of resonance energy transfer. Firstly, we scrutinize the impact of a macroscopic chiral medium enveloping the interacting molecules; secondly, we probe the effect of a chiral mediating molecule in close proximity to the system. Importantly, our findings demonstrate that chiral environments not only modulate pre-existing discriminatory effects but also introduce novel mechanisms for discrimination. ...
Aufsatz
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Nondipolar photoelectron angular distributions from fixed-in-space N₂ molecules
(2024-06-26)
We investigate experimentally and theoretically the N 1s photoionization of fixed-in-space N2 molecules at a photon energy of 880 eV. In our experiment, we employed circularly polarized synchrotron radiation for the photoionization and coincident electron and fragment-ion detection using cold target recoil ion momentum spectroscopy. The accompanying angle-resolved calculations were carried out by the multichannel single-center method and code within the frozen-core Hartree–Fock approximation. The computed emission ...
Aufsatz
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X-ray radiation damage cycle of solvated inorganic ions
(2024-05-30)
X-ray-induced damage is one of the key topics in radiation chemistry. Substantial damage is attributed to low-energy electrons and radicals emerging from direct inner-shell photoionization or produced by subsequent processes. We apply multi-electron coincidence spectroscopy to X-ray-irradiated aqueous solutions of inorganic ions to investigate the production of low-energy electrons (LEEs) in a predicted cascade of intermolecular charge- and energy-transfer processes, namely electron-transfer-mediated decay (ETMD) and ...