Aufsatz
Artikel (Publikationen im Open Access gefördert durch die UB)
Asymptotic model for shape resonance control of diatomics by intense non-resonant light: universality in the single-channel approximation
Abstract
Non-resonant light interacting with diatomics via the polarizability anisotropy couples different
rotational states and may lead to strong hybridization of the motion. The modification of shape
resonances and low-energy scattering states due to this interaction can be fully captured by an
asymptotic model, based on the long-range properties of the scattering (Crubellier et al 2015 New J.
Phys. 17 045020). Remarkably, the properties of the field-dressed shape resonances in this asymptotic
multi-channel description are found to be approximately linear in the field intensity up to fairly large
intensity. This suggests a perturbative single-channel approach to be sufficient to study the control of
such resonances by the non-resonant field. The multi-channel results furthermore indicate the
dependence on field intensity to present, at least approximately, universal characteristics. Here we
combine the nodal line technique to solve the asymptotic Schrödinger equation with perturbation
theory. Comparing our single channel results to those obtained with the full interaction potential, we
find nodal lines depending only on the field-free scattering length of the diatom to yield an
approximate but universal description of the field-dressed molecule, confirming universal behavior.
rotational states and may lead to strong hybridization of the motion. The modification of shape
resonances and low-energy scattering states due to this interaction can be fully captured by an
asymptotic model, based on the long-range properties of the scattering (Crubellier et al 2015 New J.
Phys. 17 045020). Remarkably, the properties of the field-dressed shape resonances in this asymptotic
multi-channel description are found to be approximately linear in the field intensity up to fairly large
intensity. This suggests a perturbative single-channel approach to be sufficient to study the control of
such resonances by the non-resonant field. The multi-channel results furthermore indicate the
dependence on field intensity to present, at least approximately, universal characteristics. Here we
combine the nodal line technique to solve the asymptotic Schrödinger equation with perturbation
theory. Comparing our single channel results to those obtained with the full interaction potential, we
find nodal lines depending only on the field-free scattering length of the diatom to yield an
approximate but universal description of the field-dressed molecule, confirming universal behavior.
Citation
In: New journal of physics. - London : IOP, 2015, 17, 045022, 1-15Sponsorship
Gefördert durch den Publikationsfonds der Universität KasselCollections
Publikationen (Theoretische Physik III - Quantendynamik und -kontrolle)Artikel (Publikationen im Open Access gefördert durch die UB)
Citation
@article{urn:nbn:de:hebis:34-2015070148692,
author={Crubellier, Anne and Gonzáles-Férez, Rosario and Koch, Christiane P. and Luc-Koenig, Eliane},
title={Asymptotic model for shape resonance control of diatomics by intense non-resonant light: universality in the single-channel approximation},
year={2015}
}
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2015-07-01T10:56:50Z 2015-07-01T10:56:50Z 2015 1367-2630 urn:nbn:de:hebis:34-2015070148692 http://hdl.handle.net/123456789/2015070148692 Gefördert durch den Publikationsfonds der Universität Kassel eng Urheberrechtlich geschützt https://rightsstatements.org/page/InC/1.0/ 530 Asymptotic model for shape resonance control of diatomics by intense non-resonant light: universality in the single-channel approximation Aufsatz Non-resonant light interacting with diatomics via the polarizability anisotropy couples different rotational states and may lead to strong hybridization of the motion. The modification of shape resonances and low-energy scattering states due to this interaction can be fully captured by an asymptotic model, based on the long-range properties of the scattering (Crubellier et al 2015 New J. Phys. 17 045020). Remarkably, the properties of the field-dressed shape resonances in this asymptotic multi-channel description are found to be approximately linear in the field intensity up to fairly large intensity. This suggests a perturbative single-channel approach to be sufficient to study the control of such resonances by the non-resonant field. The multi-channel results furthermore indicate the dependence on field intensity to present, at least approximately, universal characteristics. Here we combine the nodal line technique to solve the asymptotic Schrödinger equation with perturbation theory. Comparing our single channel results to those obtained with the full interaction potential, we find nodal lines depending only on the field-free scattering length of the diatom to yield an approximate but universal description of the field-dressed molecule, confirming universal behavior. open access In: New journal of physics. - London : IOP, 2015, 17, 045022, 1-15 Crubellier, Anne Gonzáles-Férez, Rosario Koch, Christiane P. Luc-Koenig, Eliane doi:10.1088/1367-2630/17/4/045022
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