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Dissertation
Energy transfer in free-standing van der Waals heterostructures after optical excitation
(2019)
The wide range of layered van der Waals materials is interesting due to its plenty of deviating characteristics. The structure of all these materials is built from covalently joined layers, which are stacked by van der Waals forces. Aside from this structural similarity the specific characteristics spread out in a variety of electronic and optical properties. The electronic properties of layered materials vary from pure insulators to metallic conductors and can even depend on the number of layers. In the work presented ...
Dissertation
Ab-initio analysis of the structural response of solids after femtosecond-laser-pulse excitation
(2019)
After an intense femtosecond-laser excitation extreme non-equilibrium conditions are induced in materials. The high photon density in such an ultrashort-laser pulse interacts directly with the electronic system of the material. By absorbing the photon energy the electrons are excited in high energy states, where they form a non-equilibrium distribution shortly after the excitation. Due to fast electron-electron scattering and cascading processes equilibrates the electronic system within several femtoseconds to a ...
Aufsatz
Exploiting non-Markovianity for quantum control
(Nature Publishing Group, 2015)
Quantum technology, exploiting entanglement and the wave nature of matter, relies on the ability to accurately control quantum systems. Quantum control is often compromised by the interaction of the system with its environment since this causes loss of amplitude and phase. However, when the dynamics of the open quantum system is non-Markovian, amplitude and phase flow not only from the system into the environment but also back. Interaction with the environment is then not necessarily detrimental. We show that the ...
Dissertation
Investigations on Diamond Thin Films as Implant Coating and Biosensing Platform
(2021)
Diamond is researched in biological context for decades. Fundamental research has established diamond as a material that combines a pronounced compatibility with biological entities and resilience against even the harshest chemical and physical conditions. The present dissertation strives to improve the abilities of diamond in this matter even further by utilizing methods of nanostructuring and biochemical functionalization. Numerous characterization methods are used to monitor each step in detail and to evaluate the ...
Aufsatz
Vesicle motion during sustained exocytosis in chromaffin cells
(PLoS, 2015)
Chromaffin cells release catecholamines by exocytosis, a process that includes vesicle docking, priming and fusion. Although all these steps have been intensively studied, some aspects of their mechanisms, particularly those regarding vesicle transport to the active sites situated at the membrane, are still unclear. In this work, we show that it is possible to extract information on vesicle motion in Chromaffin cells from the combination of Langevin simulations and amperometric measurements. We developed a numerical ...
Dissertation
Organische Magnetooptoelektronik
(2014-09-25)
Im Rahmen der Organischen Optoelektronik wird der Weg vom Molekül zum Bauteil als Wertschöpfungskette verstanden, deren Kernziele wissenschaftlicher Erkenntnisfortschritt und Produktanwendungen sind. Eine besonders vielversprechende Möglichkeit diese Entwicklung auch in Zukunft erfolgreich und innovativ fortführen zu können, eröffnet sich durch das Einbeziehen magnetosensitiver Prozesse. Spinzustände werden als zusätzliche Regelgröße verstanden, die es erlauben, optoelektronische Abläufe zu optimieren und neuartige ...
Dissertation
Electronic Theory of the Magnetic Order, Anisotropy and Reversal Processes in Rolled-Up Stripes and Thin Films
(2022)
A comprehensive multiscale approach consisting of a combination of state of the art, first principles quantum theory and the flexible statistical methodologies of complex systems is applied in order to achieve a detailed microscopic understanding of the magnetic properties of rolled-up transition-metal [TM] ultrathin films and stripes. A quantum electronic investigations of the effective interactions between the local magnetic moments is performed as a function of composition and rolling radius R including the limit ...
Dissertation
Raumwinkeloptimierte Elektron-Photon Koinzidenzmessungen nach der Anregung mit Synchrotronstrahlung unter Verwendung zeitlich verschieden strukturierter Füllmuster des Speicherrings
(2021-05)
Für die Untersuchung von Relaxationspfaden von angeregten mikroskopischen Systemen nehmen Messmethoden eine zentrale Rolle ein, bei denen emittierte Teilchen so gemessen werden, dass eine physikalische Korrelation zwischen Ihnen nachgewiesen werden kann. Denn nur durch den Nachweis dieser Korrelationen ist es bei stark verzweigten und sich unter Umständen kreuzenden Relaxationspfaden, diese Pfade eindeutig nachzuverfolgen.
Diese sogenannten Koinzidenzmessungen werden seit ihren ersten Anwendungen in den 1920er Jahren ...